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"This Old Heart of Mine (Is Weak for You)" was a successful hit single for The Isley Brothers in 1966, during their brief tenure on Motown's Tamla label. Written by Motown's main songwriting team Holland-Dozier-Holland alongside Sylvia Moy, "This Old Heart of Mine", produced by Brian Holland and Lamont Dozier, was originally intended for The Supremes (who later recorded their own version for their Supremes A' Go-Go album).

Featuring Ronald Isley on lead vocal, "This Old Heart of Mine" peaked at #12 on the Billboard Hot 100, and at #6 on the Billboard R&B Singles chart. The single was the group's only major hit while on Motown, and in 1969 the Isleys left Motown to restart their own T-Neck label. During the same year, Tammi Terrell recorded and released the song as a part of her Irresistible album. In 1976, Rod Stewart released a remake of this song that met with some success. Twenty-four years after the original recording, Ronald Isley and Rod Stewart released a Top 10 duet version of the song in 1990 that reached #10 on the US Billboard Hot 100 chart and spent five weeks at #1 on the US adult contemporary chart. The Dutch girl group Luv' recorded a dance cover version of "This Old Heart of Mine" in 1992.



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